Principles of Nonlinear Optical Spectroscopy

Author: Shaul Mukamel
Publisher: Oxford University Press on Demand
ISBN: 9780195132915
Format: PDF, ePub, Mobi
Download Now
One of the obstacles facing researchers in nonlinear optical spectroscopy is the flood of experiemtnal techniques and terminologies, which create a serious language barrier. This book presents a systematic and uifying viewpoint for a wide class of techniques.

Two Dimensional Optical Spectroscopy

Author: Minhaeng Cho
Publisher: CRC Press
ISBN: 9781420084306
Format: PDF, ePub
Download Now
Two-Dimensional Optical Spectroscopy discusses the principles and applications of newly emerging two-dimensional vibrational and optical spectroscopy techniques. It provides a detailed account of basic theory required for an understanding of two-dimensional vibrational and electronic spectroscopy. It also bridges the gap between the formal development of nonlinear optical spectroscopy and the application of the theory to explain experimental results. Focusing on time-domain spectroscopy, the book presents detailed discussions on the underlying physics and interpretation methods of a variety of two-dimensional optical spectroscopic methods. It illustrates how novel diagrammatic techniques are useful in graphically describing the associated nonlinear optical transition pathways and involved population or coherence evolutions. The author also explains the basics of quantum dynamics and time-dependent perturbation theories that are required in describing nonlinear optical processes. From the development of the theory to novel applications, this book covers a gamut of topics in this field, including perturbation theory, coherent Raman scattering, pump-probe spectroscopy, photon echo spectroscopy, IR-visible four-wave mixing, and linear and nonlinear optical activity spectroscopy. It shows how to apply the recently developed tools of vibrational and electronic spectroscopy in two dimensions.

Quantum Metrology with Photoelectrons

Author: Paul Hockett
Publisher: Morgan & Claypool Publishers
ISBN: 1681746883
Format: PDF, ePub, Mobi
Download Now
Since the turn of the century, the increasing availability of photoelectron imaging experiments, along with the increasing sophistication of experimental techniques, and the availability of computational resources for analysis and numerics, has allowed for significant developments in such photoelectron metrology. Quantum Metrology with Photoelectrons, Volume 2: Applications and Advances discusses the fundamental concepts along with recent and emerging applications. Volume 2 explores the applications and development of quantum metrology schemes based on photoelectron measurements. The author begins with a brief historical background on "complete" photoionization experiments, followed by the details of state reconstruction methodologies from experimental measurements. Three specific applications of quantum metrology schemes are discussed in detail. In addition, the book provides advances, future directions, and an outlook including (ongoing) work to generalise these schemes and extend them to dynamical many-body systems. Volume 2 will be of interest to readers wishing to see the (sometimes messy) details of state reconstruction from photoelectron measurements as well as explore the future prospects for this class of metrology.

Ultrafast Dynamics at the Nanoscale

Author: Stefan Haacke
Publisher: CRC Press
ISBN: 1315340925
Format: PDF, Mobi
Download Now
Ultrafast Dynamics at the Nanoscale provides a combined experimental and theoretical insight into the molecular-level investigation of light-induced quantum processes in biological systems and nanostructured (bio)assemblies. Topics include DNA photostability and repair, photoactive proteins, biological and artificial light-harvesting systems, plasmonic nanostructures, and organic photovoltaic materials, whose common denominator is the key importance of ultrafast quantum effects at the border between the molecular scale and the nanoscale. The functionality and control of these systems have been under intense investigation in recent years in view of developing a detailed understanding of ultrafast nanoscale energy and charge transfer, as well as fostering novel technologies based on sustainable energy resources. Both experiment and theory have made big strides toward meeting the challenge of these truly complex systems. This book, thus, introduces the reader to cutting-edge developments in ultrafast nonlinear optical spectroscopies and the quantum dynamical simulation of the observed dynamics, including direct simulations of two-dimensional optical experiments. Taken together, these techniques attempt to elucidate whether the quantum coherent nature of ultrafast events enhances the efficiency of the relevant processes and where the quantum–classical boundary sets in, in these high-dimensional biological and material systems. The chapters contain well-illustrated accounts of the authors’ research work, including didactic introductory material, and address a multidisciplinary audience from chemistry, physics, biology, and materials sciences. The book is, therefore, a must-have for graduate- and postgraduate-level researchers who wish to learn about molecular nanoscience from a combined spectroscopic and theoretical viewpoint.

Metal Clusters and Nanoalloys

Author: Marcelo Mario Mariscal
Publisher: Springer Science & Business Media
ISBN: 1461436435
Format: PDF, Kindle
Download Now
Metallic nanoparticles hold promise for their potential applications in a wide array of disciplines ranging from materials science to medicine. This book brings the power of theoretical methods to an audience of experimentalists, and explicates the simulation of metallic clusters and nanoparticles. It begins with a summary of the current state of research on metallic nanoparticles, then moves on to the current state of the art in theory of metallic nanoparticldes, and then explains why and how these tools help experimentalists. Contributions are provided by renowned experts in the field from across the world.

Analysis and Control of Ultrafast Photoinduced Reactions

Author: Oliver Kühn
Publisher: Springer Science & Business Media
ISBN: 3540680373
Format: PDF
Download Now
Dynamical processes in molecules like bond shaking, breaking or making c- monlytakeplaceonatimescalefromthepico-downtothefemtosecondrange. Theadventofequallyfastlasersourcesandreal-timeobservationschemeslike pump-probe spectroscopy has facilitated the direct insight into such processes wheninitiatedbylight. Inparallelthedevelopmentofadvancedcomputational methods treating the dynamics of photoexcited molecular systems allowed a convergence between theoretical description and experimental observation of such ultrafast dynamical processes. Consequently, the idea emerged, not only to analyze, but also to control molecular dynamics in real time by adequately designed light ?elds. Stimulated by theoretical concepts for in?uencing the motion of molecular wave packets by means of simple few-parameter elect- magnetic ?eld sequences, experiments were driven toward a practical reali- tion of arbitrarily shaped laser pulses. This development culminated in the active feedback control of even complex systems. In addition this o?ers the unique possibility not only to determine the outcome of chemical reactions, butalsotoretrievespeci?cinformationaboutthechosendynamicalpathways, that is, to perform analysis by control. This book illustrates a vital research ?eld by covering a broad spectrum of molecular systems with growing complexity while demonstrating at the same time the convergence of experimental and theoretical approaches. After a g- eral introduction in Chapter 1, Chapter 2 starts with small isolated molecules in the unperturbed environment of the gas phase and Chapter 3 proceeds to more complex systems, but still in vacuum. A higher level of complexity is then reached in Chapter 4 where small molecules in a rare gas matrices are discussed serving as prototype examples for condensed phase dynamics.

Concepts and Methods of 2D Infrared Spectroscopy

Author: Peter Hamm
Publisher: Cambridge University Press
ISBN: 1139497073
Format: PDF, Docs
Download Now
2D infrared (IR) spectroscopy is a cutting-edge technique, with applications in subjects as diverse as the energy sciences, biophysics and physical chemistry. This book introduces the essential concepts of 2D IR spectroscopy step-by-step to build an intuitive and in-depth understanding of the method. This unique book introduces the mathematical formalism in a simple manner, examines the design considerations for implementing the methods in the laboratory, and contains working computer code to simulate 2D IR spectra and exercises to illustrate involved concepts. Readers will learn how to accurately interpret 2D IR spectra, design their own spectrometer and invent their own pulse sequences. It is an excellent starting point for graduate students and researchers new to this exciting field. Computer codes and answers to the exercises can be downloaded from the authors' website, available at www.cambridge.org/9781107000056.

The Physics and Applications of Photorefractive Materials

Author: L. Solymar
Publisher: Clarendon Press
ISBN: 9780191589102
Format: PDF
Download Now
Photorefractive materials combine photoconductive and electro-optic properties: light affects their electrical conductivity; their optical properties (refractive index, etc.) are affected by applied electric fields. The aim of this book is to cover the vast range of phenomena occurring in Photorefractive Materials. For Physicists it is part of the fashionable subject of Nonlinear Optics. Engineers tend to place it as part of optoelectronics promising a variety of new devices. This book summarizes the results of 28 years of research in a manner that would appeal both to the beginner (a graduate student who has just entered the field) and to the expert (who might have done research on some aspect of the subject for a decade or more). It is in three parts. Part I serves as an introduction with emphasis on physical principles and simple mathematical models. Part II is a comprehensive account of all the major advances. Its main merit is the organization of the material accompanied by a detailed list of references. Part III is concerned with the enormous range of potential applications.

Methods in Theoretical Quantum Optics

Author: Stephen Barnett
Publisher: Oxford University Press
ISBN: 9780198563617
Format: PDF, ePub
Download Now
This work presents the mathematical methods widely used by workers in the field of quantum optics. It deals with the physical assumptions which lead to the models and approximations employed, but the main purpose of the text is to give a firm grounding in those techniques needed to derive analytical solutions to problems.

Atomic and Laser Spectroscopy

Author: Alan Corney
Publisher: Oxford University Press
ISBN: 0199211450
Format: PDF, ePub, Mobi
Download Now
This book discusses many advances in optical physics and is intended mainly for experimentalists. The interaction of electromagnetic radiation with free atoms is introduced using classical or semi-classical calculations wherever possible. Topics discussed include the spontaneous emission of radiation, and atomic beam magnetic resonance experiments.